Acetaldehyde removal and increased H2/CO gas yield from biomass gasification over metal-loaded Kraft lignin char catalyst.
Identifieur interne : 000B50 ( Main/Exploration ); précédent : 000B49; suivant : 000B51Acetaldehyde removal and increased H2/CO gas yield from biomass gasification over metal-loaded Kraft lignin char catalyst.
Auteurs : Ki Hoon Kim [Corée du Sud] ; Abid Farooq [Corée du Sud] ; Min Young Song [Corée du Sud] ; Sang-Chul Jung [Corée du Sud] ; Ki-Joon Jeon [Corée du Sud] ; Jihyeon Song [Corée du Sud] ; Chang Hyun Ko [Corée du Sud] ; Jungho Jae [Corée du Sud] ; Young-Kwon Park [Corée du Sud]Source :
- Journal of environmental management [ 1095-8630 ] ; 2019.
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Abstract
Acetaldehyde removal tests were performed to compare the catalytic activity of the Kraft lignin char (KC), KOH-treated Kraft lignin char (KKC), and activated carbon (AC) along with their impregnation with Mn in a plasma reactor. The gasification characteristics (syngas content, and H2/CO ratio) of yellow poplar were investigated using nickel catalysts supported on KC, KKC, AC, and γ-Al2O3 in a U-type quartz reactor. KKC and Mn/KKC improved significantly the surface area and contents of O and N functional groups over the raw char. In particular, Mn/KKC showed the highest acetaldehyde-removal efficiency. The catalytic activity of Ni-impregnated KC, KKC, AC, and γ-Al2O3 decreased in the order of Ni/KKC > Ni/AC > Ni/KC > Ni/γ-Al2O3 for the gas yield and Ni/γ-Al2O3 >Ni/KC > Ni/AC >Ni/KKC for the oil yield, respectively. The Ni/KKC provides a more conducive environment for gasification, resulting in larger amounts of syngas (H2 and CO) in the product gases. Moreover, Ni impregnated with char may be the most inexpensive and effective solution for achieving maximum tar reduction and syngas generation.
DOI: 10.1016/j.jenvman.2018.11.054
PubMed: 30496962
Affiliations:
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xml:lang="en">Acetaldehyde removal and increased H<sub>2</sub>/CO gas yield from biomass gasification over metal-loaded Kraft lignin char catalyst.</title><author><name sortKey="Kim, Ki Hoon" sort="Kim, Ki Hoon" uniqKey="Kim K" first="Ki Hoon" last="Kim">Ki Hoon Kim</name><affiliation wicri:level="1"><nlm:affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>School of Environmental Engineering, University of Seoul, Seoul 02504</wicri:regionArea><placeName><settlement type="city">Séoul</settlement><region type="capital">Région capitale de Séoul</region></placeName></affiliation></author><author><name sortKey="Farooq, Abid" sort="Farooq, Abid" uniqKey="Farooq A" first="Abid" last="Farooq">Abid Farooq</name><affiliation wicri:level="1"><nlm:affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>School of Environmental Engineering, University of Seoul, Seoul 02504</wicri:regionArea><placeName><settlement type="city">Séoul</settlement><region type="capital">Région capitale de Séoul</region></placeName></affiliation></author><author><name sortKey="Song, Min Young" sort="Song, Min Young" uniqKey="Song M" first="Min Young" last="Song">Min Young Song</name><affiliation wicri:level="1"><nlm:affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>School of Environmental Engineering, University of Seoul, Seoul 02504</wicri:regionArea><placeName><settlement type="city">Séoul</settlement><region type="capital">Région capitale de Séoul</region></placeName></affiliation></author><author><name sortKey="Jung, Sang Chul" sort="Jung, Sang Chul" uniqKey="Jung S" first="Sang-Chul" last="Jung">Sang-Chul Jung</name><affiliation wicri:level="1"><nlm:affiliation>Department of Environmental Engineering, Sunchon National University, Suncheon 57922, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>Department of Environmental Engineering, Sunchon National University, Suncheon 57922</wicri:regionArea><wicri:noRegion>Suncheon 57922</wicri:noRegion></affiliation></author><author><name sortKey="Jeon, Ki Joon" sort="Jeon, Ki Joon" uniqKey="Jeon K" first="Ki-Joon" last="Jeon">Ki-Joon Jeon</name><affiliation wicri:level="1"><nlm:affiliation>Department of Environmental Engineering, Inha University, Incheon 22212, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>Department of Environmental Engineering, Inha University, Incheon 22212</wicri:regionArea><wicri:noRegion>Incheon 22212</wicri:noRegion></affiliation></author><author><name sortKey="Song, Jihyeon" sort="Song, Jihyeon" uniqKey="Song J" first="Jihyeon" last="Song">Jihyeon Song</name><affiliation wicri:level="1"><nlm:affiliation>Department of Civil and Environmental Engineering, Sejong University, Seoul, 05006, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>Department of Civil and Environmental Engineering, Sejong University, Seoul, 05006</wicri:regionArea><wicri:noRegion>05006</wicri:noRegion></affiliation></author><author><name sortKey="Ko, Chang Hyun" sort="Ko, Chang Hyun" uniqKey="Ko C" first="Chang Hyun" last="Ko">Chang Hyun Ko</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical Engineering, Chonnam National University, Gwangju, 61186, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>School of Chemical Engineering, Chonnam National University, Gwangju, 61186</wicri:regionArea><wicri:noRegion>61186</wicri:noRegion></affiliation></author><author><name sortKey="Jae, Jungho" sort="Jae, Jungho" uniqKey="Jae J" first="Jungho" last="Jae">Jungho Jae</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Biomolecular Engineering, Pusan National University, Busan 46241, South Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>School of Chemical and Biomolecular Engineering, Pusan National University, Busan 46241</wicri:regionArea><wicri:noRegion>Busan 46241</wicri:noRegion></affiliation></author><author><name sortKey="Park, Young Kwon" sort="Park, Young Kwon" uniqKey="Park Y" first="Young-Kwon" last="Park">Young-Kwon Park</name><affiliation wicri:level="1"><nlm:affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea. Electronic address: catalica@uos.ac.kr.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>School of Environmental Engineering, University of Seoul, Seoul 02504</wicri:regionArea><placeName><settlement type="city">Séoul</settlement><region type="capital">Région capitale de Séoul</region></placeName></affiliation></author></analytic><series><title level="j">Journal of environmental management</title><idno type="eISSN">1095-8630</idno><imprint><date when="2019" type="published">2019</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Acetaldehyde (MeSH)</term><term>Biomass (MeSH)</term><term>Catalysis (MeSH)</term><term>Gases (MeSH)</term><term>Lignin (MeSH)</term><term>Metals (MeSH)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Acétaldéhyde (MeSH)</term><term>Biomasse (MeSH)</term><term>Catalyse (MeSH)</term><term>Gaz (MeSH)</term><term>Lignine (MeSH)</term><term>Métaux (MeSH)</term></keywords><keywords scheme="MESH" type="chemical" xml:lang="en"><term>Acetaldehyde</term><term>Gases</term><term>Lignin</term><term>Metals</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Biomass</term><term>Catalysis</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Acétaldéhyde</term><term>Biomasse</term><term>Catalyse</term><term>Gaz</term><term>Lignine</term><term>Métaux</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Acetaldehyde removal tests were performed to compare the catalytic activity of the Kraft lignin char (KC), KOH-treated Kraft lignin char (KKC), and activated carbon (AC) along with their impregnation with Mn in a plasma reactor. The gasification characteristics (syngas content, and H<sub>2</sub>/CO ratio) of yellow poplar were investigated using nickel catalysts supported on KC, KKC, AC, and γ-Al<sub>2</sub>O<sub>3</sub> in a U-type quartz reactor. KKC and Mn/KKC improved significantly the surface area and contents of O and N functional groups over the raw char. In particular, Mn/KKC showed the highest acetaldehyde-removal efficiency. The catalytic activity of Ni-impregnated KC, KKC, AC, and γ-Al<sub>2</sub>O<sub>3</sub> decreased in the order of Ni/KKC > Ni/AC > Ni/KC > Ni/γ-Al<sub>2</sub>O<sub>3</sub> for the gas yield and Ni/γ-Al<sub>2</sub>O<sub>3</sub> >Ni/KC > Ni/AC >Ni/KKC for the oil yield, respectively. The Ni/KKC provides a more conducive environment for gasification, resulting in larger amounts of syngas (H<sub>2</sub> and CO) in the product gases. Moreover, Ni impregnated with char may be the most inexpensive and effective solution for achieving maximum tar reduction and syngas generation.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" IndexingMethod="Automated" Owner="NLM"><PMID Version="1">30496962</PMID><DateCompleted><Year>2019</Year><Month>09</Month><Day>24</Day></DateCompleted><DateRevised><Year>2019</Year><Month>09</Month><Day>25</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1095-8630</ISSN><JournalIssue CitedMedium="Internet"><Volume>232</Volume><PubDate><Year>2019</Year><Month>Feb</Month><Day>15</Day></PubDate></JournalIssue><Title>Journal of environmental management</Title><ISOAbbreviation>J Environ Manage</ISOAbbreviation></Journal><ArticleTitle>Acetaldehyde removal and increased H<sub>2</sub>/CO gas yield from biomass gasification over metal-loaded Kraft lignin char catalyst.</ArticleTitle><Pagination><MedlinePgn>330-335</MedlinePgn></Pagination><ELocationID EIdType="pii" ValidYN="Y">S0301-4797(18)31319-7</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.jenvman.2018.11.054</ELocationID><Abstract><AbstractText>Acetaldehyde removal tests were performed to compare the catalytic activity of the Kraft lignin char (KC), KOH-treated Kraft lignin char (KKC), and activated carbon (AC) along with their impregnation with Mn in a plasma reactor. The gasification characteristics (syngas content, and H<sub>2</sub>/CO ratio) of yellow poplar were investigated using nickel catalysts supported on KC, KKC, AC, and γ-Al<sub>2</sub>O<sub>3</sub> in a U-type quartz reactor. KKC and Mn/KKC improved significantly the surface area and contents of O and N functional groups over the raw char. In particular, Mn/KKC showed the highest acetaldehyde-removal efficiency. The catalytic activity of Ni-impregnated KC, KKC, AC, and γ-Al<sub>2</sub>O<sub>3</sub> decreased in the order of Ni/KKC > Ni/AC > Ni/KC > Ni/γ-Al<sub>2</sub>O<sub>3</sub> for the gas yield and Ni/γ-Al<sub>2</sub>O<sub>3</sub> >Ni/KC > Ni/AC >Ni/KKC for the oil yield, respectively. The Ni/KKC provides a more conducive environment for gasification, resulting in larger amounts of syngas (H<sub>2</sub> and CO) in the product gases. Moreover, Ni impregnated with char may be the most inexpensive and effective solution for achieving maximum tar reduction and syngas generation.</AbstractText><CopyrightInformation>Copyright © 2018 Elsevier Ltd. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Kim</LastName><ForeName>Ki Hoon</ForeName><Initials>KH</Initials><AffiliationInfo><Affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Farooq</LastName><ForeName>Abid</ForeName><Initials>A</Initials><AffiliationInfo><Affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Song</LastName><ForeName>Min Young</ForeName><Initials>MY</Initials><AffiliationInfo><Affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Jung</LastName><ForeName>Sang-Chul</ForeName><Initials>SC</Initials><AffiliationInfo><Affiliation>Department of Environmental Engineering, Sunchon National University, Suncheon 57922, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Jeon</LastName><ForeName>Ki-Joon</ForeName><Initials>KJ</Initials><AffiliationInfo><Affiliation>Department of Environmental Engineering, Inha University, Incheon 22212, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Song</LastName><ForeName>JiHyeon</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>Department of Civil and Environmental Engineering, Sejong University, Seoul, 05006, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Ko</LastName><ForeName>Chang Hyun</ForeName><Initials>CH</Initials><AffiliationInfo><Affiliation>School of Chemical Engineering, Chonnam National University, Gwangju, 61186, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Jae</LastName><ForeName>Jungho</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>School of Chemical and Biomolecular Engineering, Pusan National University, Busan 46241, South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Park</LastName><ForeName>Young-Kwon</ForeName><Initials>YK</Initials><AffiliationInfo><Affiliation>School of Environmental Engineering, University of Seoul, Seoul 02504, South Korea. Electronic address: catalica@uos.ac.kr.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2018</Year><Month>11</Month><Day>27</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>J Environ Manage</MedlineTA><NlmUniqueID>0401664</NlmUniqueID><ISSNLinking>0301-4797</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D005740">Gases</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D008670">Metals</NameOfSubstance></Chemical><Chemical><RegistryNumber>8068-05-1</RegistryNumber><NameOfSubstance UI="C076151">Kraft lignin</NameOfSubstance></Chemical><Chemical><RegistryNumber>9005-53-2</RegistryNumber><NameOfSubstance UI="D008031">Lignin</NameOfSubstance></Chemical><Chemical><RegistryNumber>GO1N1ZPR3B</RegistryNumber><NameOfSubstance UI="D000079">Acetaldehyde</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000079" MajorTopicYN="Y">Acetaldehyde</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D018533" MajorTopicYN="N">Biomass</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002384" MajorTopicYN="N">Catalysis</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D005740" MajorTopicYN="Y">Gases</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D008031" MajorTopicYN="N">Lignin</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D008670" MajorTopicYN="N">Metals</DescriptorName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Acetaldehyde removal</Keyword><Keyword MajorTopicYN="N">Biomass</Keyword><Keyword MajorTopicYN="N">Catalyst</Keyword><Keyword MajorTopicYN="N">Gasification</Keyword><Keyword MajorTopicYN="N">Kraft lignin char</Keyword><Keyword MajorTopicYN="N">Plasma</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2018</Year><Month>09</Month><Day>17</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2018</Year><Month>10</Month><Day>28</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2018</Year><Month>11</Month><Day>15</Day></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2018</Year><Month>11</Month><Day>30</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2019</Year><Month>9</Month><Day>26</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2018</Year><Month>11</Month><Day>30</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">30496962</ArticleId><ArticleId IdType="pii">S0301-4797(18)31319-7</ArticleId><ArticleId IdType="doi">10.1016/j.jenvman.2018.11.054</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>Corée du Sud</li></country><region><li>Région capitale de Séoul</li></region><settlement><li>Séoul</li></settlement></list><tree><country name="Corée du Sud"><region name="Région capitale de Séoul"><name sortKey="Kim, Ki Hoon" sort="Kim, Ki Hoon" uniqKey="Kim K" first="Ki Hoon" last="Kim">Ki Hoon Kim</name></region><name sortKey="Farooq, Abid" sort="Farooq, Abid" uniqKey="Farooq A" first="Abid" last="Farooq">Abid Farooq</name><name sortKey="Jae, Jungho" sort="Jae, Jungho" uniqKey="Jae J" first="Jungho" last="Jae">Jungho Jae</name><name sortKey="Jeon, Ki Joon" sort="Jeon, Ki Joon" uniqKey="Jeon K" first="Ki-Joon" last="Jeon">Ki-Joon Jeon</name><name sortKey="Jung, Sang Chul" sort="Jung, Sang Chul" uniqKey="Jung S" first="Sang-Chul" last="Jung">Sang-Chul Jung</name><name sortKey="Ko, Chang Hyun" sort="Ko, Chang Hyun" uniqKey="Ko C" first="Chang Hyun" last="Ko">Chang Hyun Ko</name><name sortKey="Park, Young Kwon" sort="Park, Young Kwon" uniqKey="Park Y" first="Young-Kwon" last="Park">Young-Kwon Park</name><name sortKey="Song, Jihyeon" sort="Song, Jihyeon" uniqKey="Song J" first="Jihyeon" last="Song">Jihyeon Song</name><name sortKey="Song, Min Young" sort="Song, Min Young" uniqKey="Song M" first="Min Young" last="Song">Min Young Song</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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